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Effect of short-term atrazine addition on the performance of an anaerobic/anoxic/oxic process

Changyong WU, Xiaoling LI, Zhiqiang CHEN, Yongzhen PENG,

《环境科学与工程前沿（英文）》 2010年 第4卷 第2期   页码 150-156 doi: 10.1007/s11783-010-0020-9

摘要： In this study, an anaerobic/anoxic/oxic (AO) wastewater treatment process was implemented to treat domestic wastewater with short-term atrazine addition. The results provided an evaluation on the effects of an accidental pollution on the operation of a wastewater treatment plant (WWTP) in relation to Chemical Oxygen Demand (COD) and biological nutrient removal. Domestic wastewater with atrazine addition in 3 continuous days was treated when steady biological nutrient removal was achieved in the AO process. The concentrations of atrazine were 15, 10, and 5mg·L on days 1, 2 and 3, respectively. The results showed that atrazine addition did not affect the removal of COD. The specific NH NO reduction rate decreased slightly due to the short-term atrazine addition. However, it did not affect the nitrogen removal due to the high nitrification and denitrification capacity of the system. Total nitrogen (TN) removal was steady, and more than 70% was removed during the period studied. The phosphorus removal rate was not affected by the short-term addition of atrazine under the applied experimental conditions. However, more poly-hydroxy-alkanoate (PHA) was generated and utilized during atrazine addition. The results of the oxygen uptake rate (OUR) showed that the respiration of nitrifiers decreased significantly, while the activity of carbon utilizers had no obvious change with the atrazine addition. Atrazine was not removed with the AO process, even via absorption by the activated sludge in the process of the short-term addition of atrazine.

关键词： biological nutrient removal     atrazine     anaerobic/anoxic/oxic (A2O) process     oxygen demand removal     oxygen uptake rate (OUR)    

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Reduction of wastewater toxicity and change of microbial community in a hydrolysis acidification reactor pre-treating trimethylolpropane wastewater

Xin Xing, Yin Yu, Hongbo Xi, Guangqing Song, Yajiao Wang, Jiane Zuo, Yuexi Zhou

《环境科学与工程前沿（英文）》 2018年 第12卷 第6期 doi: 10.1007/s11783-018-1055-6

摘要：

HAP was verified to reduce the toxicity of TMP wastewater effectively.

Actual TMP wastewater was fed in HAP with different dilution ratios for 240 days.

Formaldehyde, 2-ethylacrolein, TMP and 2-ethylhexanol were all greatly removed.

Firmicutes became the dominant phylum (the abundance increased to 57.08%).

关键词： Trimethylolpropane wastewater     Hydrolysis acidification process     Toxicity     Oxygen uptake rate     16S rDNA    

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the addition of organic carbon sources on nitrous oxide emission in anaerobic-aerobic (low dissolved oxygen

Hongjing LI, Xiurong CHEN, Yinguang CHEN

《环境科学与工程前沿（英文）》 2010年 第4卷 第4期   页码 490-499 doi: 10.1007/s11783-010-0248-4

摘要： The effect of additional organic carbon sources on the production of nitrous oxide (N O) in anaerobic-aerobic (low dissolved oxygen) real wastewater treatment system was investigated. In this paper, three laboratory-scale sequencing batch reactors (SBRs) (SBR-1, SBR-2 and SBR-3) were operating under an anaerobic-aerobic (low dissolved oxygen, 0.15–0.45 mg·L ) configuration. The SBRs were ‘long-term cultured’ respectively with a single municipal wastewater sample, sodium acetate, and a waste-activated sludge alkaline fermentation liquid as the additional carbon sources of real wastewater. Off-gas analysis showed that N O was emitted into the atmosphere during the aerobic (low dissolved oxygen) period in the three SBRs, and the order of N O emission rate was SBR-2>SBR-1>SBR-3. It was observed that the higher poly-β-hydroxyvalerate fraction of polyhydroxyalkanoates, the lower glycogen transformation and less nitrite accumulation was in SBR-3, while the opposite behavior was observed in SBR-2. Further research indicated that the interaction of the factors above potentially affected the N O emission in the anaerobic-aerobic (low dissolved oxygen) system.

关键词： anaerobic-aerobic (low dissolved oxygen)     nitrous oxide (N2O) emitting rate     municipal wastewater     waste activated sludge     alkaline fermentation liquid    

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Comments on “Prediction on CO uptake of recycled aggregate concrete”, Frontiers of Structural and Civil

《结构与土木工程前沿（英文）》 2021年 第15卷 第6期   页码 1504-1506 doi: 10.1007/s11709-021-0782-0

摘要： A methodology to compute the CO2 uptake of recycled aggregate concrete is proposed in the commented paper. Besides some typos in several formulas, it is found that the approach to estimate the specific surface area of the recycled aggregates is not correct. This issue has some impact in the conclusions of the commented paper. Therefore, aiming to improve the understanding, accuracy and findings of the commented paper, an alternative approach to estimate the specific surface area of the recycled aggregates, as well as an erratum of the formulas and revised conclusions are suggested.
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Organic and inorganic phosphorus uptake by bacteria in a plug-flow microcosm

Jinbo ZHAO, Xuehua LIU

《环境科学与工程前沿（英文）》 2013年 第7卷 第2期   页码 173-184 doi: 10.1007/s11783-013-0494-3

摘要： Phosphorus (P) is a vital nutrient for sustaining natural water productivity. Both particulate and dissolved forms of organic and inorganic P are potentially important sources of bioavailable P for primary and secondary producers. A microcosm system to imitate the bacterial community in Plym river sediment and pore water is described and bacterial uptake rates for inorganic and organic phosphorus are presented in this paper. The aim of this study was to investigate the uptake of two organic phosphorus compounds (phytic acid and D-glucose-6-phosphate) by freshwater bacteria. The bioreactors comprise glass columns packed with two types of small glass beads on which bacterial biofilm can develop. The glass beads with different porosity were introduced to simulate River SPM. The selected P compounds spiked into the inflow of the microcosm, and measured the step change of P concentration in the outflow to investigate the behavior of bacterial uptake of nutrients. The results showed that organic phosphorus was converted into inorganic phosphorus but the conversion rate depended on the type of phosphorus species. One experiment suggested that phytic acid (refractory) could displace phosphate from the biofilm surface; the other experiment showed that D-glucose-6-phosphate (labile) could be hydrolysed and utilized easily by the bacteria. The results also suggested that bacteria might break down the C-P bonds to utilize the carbon. Further experiments should investigate the effect of varying the C:N:P ratio in the microcosm system to determine which nutrient limits bacteria uptake.

关键词： organic phosphorus     bacteria     uptake    

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The implications of planting mode on cadmium uptake and remobilization in rice: Field experiments across

《环境科学与工程前沿（英文）》 2021年 第15卷 第6期 doi: 10.1007/s11783-021-1431-5

摘要：

•Direct seeding (DS) method led to more distributed Cd in aerial parts of rice.

关键词： Cadmium     Genotypes     Growth stages     Micro X-ray fluorescence     Planting mode    

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Denitrification and phosphorus uptake by DPAOs using nitrite as an electron acceptor by step-feed strategies

Bin MA, Shuying WANG, Guibing ZHU, Shijian GE, Junmin WANG, Nanqi Ren, Yongzhen PENG

《环境科学与工程前沿（英文）》 2013年 第7卷 第2期   页码 267-272 doi: 10.1007/s11783-012-0439-2

摘要： Denitrifying phosphorus accumulating organisms (DPAOs) using nitrite as an electron acceptor can reduce more energy. However, nitrite has been reported to have an inhibition on denitrifying phosphorus removal. In this study, the step-feed strategy was proposed to achieve low nitrite concentration, which can avoid or relieve nitrite inhibition. The results showed that denitrification rate, phosphorus uptake rate and the ratio of the phosphorus uptaken to nitrite denitrified (anoxic P/N ratio) increased when the nitrite concentration was 15 mg·L after step-feeding nitrite. The maximum denitrification rate and phosphorus uptake rate was 12.73 mg and 18.75 mg , respectively. These rates were higher than that using nitrate (15 mg·L ) as an electron acceptor. The maximum anoxic P/N ratio was 1.55 mg . When the nitrite concentration increased from 15 to 20 mg after addition of nitrite, the anoxic phosphorus uptake was inhibited by 64.85%, and the denitrification by DPAOs was inhibited by 61.25%. Denitrification rate by DPAOs decreased gradually when nitrite (about 20 mg·L ) was added in the step-feed SBR. These results indicated that the step-feed strategy can be used to achieve denitrifying phosphorus removal using nitrite as an electron acceptor, and nitrite concentration should be maintained at low level (<15 mg·L in this study).

关键词： denitrifying phosphate accumulating organisms (DPAOs)     denitrification     phosphorus uptake     nitrite     step-feed     enhanced biological phosphorus removal    

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Effects of nitrite on phosphate uptake in anaerobic-oxic process

LI Jie, XIONG Biyong, ZHANG Shude, YANG Hong, ZHANG Jie

《环境科学与工程前沿（英文）》 2007年 第1卷 第1期   页码 39-42 doi: 10.1007/s11783-007-0007-3

摘要： An anaerobic-oxic (A/O) biological phosphorus removal reactor was operated to study the effect of nitrite on phosphate uptake. The phosphorus uptake profile was determined under different operating conditions. The results indicated that in addition to oxygen and nitrate (DPB, nitrate denitrifying phosphorus removal), to some extent, nitrite could also serve as an electron acceptor to achieve nitrite denitrifying phosphorus removal (DPB). The quantity and rate of phosphorus uptake of DPB, however, were evidently lower than that of DPB The experiment results revealed that nitrite would bring toxic action to phosphate-accumulating organisms (PAOs) when NO-N"e93.7 mg/L. The nitrite existing in the anoxic reactor made no difference to the quantity and rate of denitrifying phosphorus removal, but it could reduce the consumption of nitrate. Moreover, the data showed that the aerobic phosphate uptake of DPB was lower than that of anaerobic phosphorus-released sludge in a traditional A/O process. However, there was not much difference between these two kinds of sludge in terms of the total phosphorus uptake quantity and the effluent quality.

关键词： effluent     PAOs     experiment     phosphate-accumulating     phosphorus removal    

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Design of nanocarriers for efficient cellular uptake and endosomal release of small molecule and nucleic

Vaibhav Mundra, Ram I. Mahato

《化学科学与工程前沿（英文）》 2014年 第8卷 第4期   页码 387-404 doi: 10.1007/s11705-014-1457-3

摘要： There are many challenges in developing efficient and target specific delivery systems of small molecule and nucleic acid drugs. Cell membrane presents one of the major barriers for the penetration of hydrophilic macromolecules across the plasma membrane. Nanocarriers have been designed to enhance their cellular uptake via endocytosis but following their cellular uptake, endosomal escape is the rate limiting step which restricts the value associated with the enhanced uptake by nanocarriers. Viruses are an excellent model for efficient cytosolic delivery by nanocarriers. Viruses exploit intracellular cues to release the genome to cytosol. In this review, we first discuss different endocytic uptake pathways and endosomal escape mechanisms. We then summarize the existing tools for studying the intracellular trafficking of nanocarriers. Finally, we highlight the important design elements of recent virus-based nanocarriers for efficient cellular uptake and endosomal escape.

关键词： nanocarrier     cellular uptake     endosomal release     nucleic acid drug    

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Heterometallic cluster-based organic frameworks as highly active electrocatalysts for oxygen reductionand oxygen evolution reaction: a density functional theory study

《化学科学与工程前沿（英文）》 2023年 第17卷 第5期   页码 570-580 doi: 10.1007/s11705-022-2247-y

摘要： Recently, metal–organic frameworks are one of the potential catalytic materials for electrocatalytic applications. The oxygen reduction reaction and oxygen evolution reaction catalytic activities of heterometallic cluster-based organic frameworks are investigated using density functional theory. Firstly, the catalytic activities of heterometallic clusters are investigated. Among all heterometallic clusters, Fe2Mn–Mn has a minimum overpotential of 0.35 V for oxygen reduction reaction, and Fe2Co–Co possesses the smallest overpotential of 0.32 V for oxygen evolution reaction, respectively 100 and 50 mV lower than those of Pt(111) and RuO2(110) catalysts. The analysis of the potential gap of Fe2M clusters indicates that Fe2Mn, Fe2Co, and Fe2Ni clusters possess good bifunctional catalytic activity. Additionally, the catalytic activity of Fe2Mn and Fe2Co connected through 3,3′,5,5′-azobenzenetetracarboxylate linker to form Fe2M–PCN–Fe2M is explored. Compared with Fe2Mn–PCN–Fe2Mn, Fe2Co–PCN–Fe2Co, and isolated Fe2M clusters, the mixed-metal Fe2Co–PCN–Fe2Mn possesses excellent bifunctional catalytic activity, and the values of potential gap on the Mn and Co sites of Fe2Co–PCN–Fe2Mn are 0.69 and 0.70 V, respectively. Furthermore, the analysis of the electron structure indicates that constructing a mixed-metal cluster can efficiently enhance the electronic properties of the catalyst. In conclusion, the mixed-metal cluster strategy provides a new approach to further design and synthesize high-efficiency bifunctional electrocatalysts.

关键词： bimetallic metal–organic frameworks     bifunctional electrocatalyst     density functional theory     oxygen reduction reaction     oxygen evolution reaction    

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Uptake and accumulation of multiwalled carbon nanotubes change the morphometric and biochemical characteristics

Elena SMIRNOVA, Alexander GUSEV, Olga ZAYTSEVA, Olga SHEINA, Alexey TKACHEV, Elena KUZNETSOVA, Elena LAZAREVA, Galina ONISHCHENKO, Alexey FEOFANOV, Mikhail KIRPICHNIKOV

《化学科学与工程前沿（英文）》 2012年 第6卷 第2期   页码 132-138 doi: 10.1007/s11705-012-1290-5

摘要： We have studied the effect of the engineered nanomaterial Taunit, containing multiwalled carbon nanotubes (MWCNTs), on the growth of seedlings and investigated whether affected plants uptake and accumulate MWCNTs. We found that 100 μg/mL and 1000 μg/mL of Taunit stimulated the growth of roots and stems, and enhanced the peroxidase activity in these parts of plants. Microscopy studies showed the presence of MWCNTs in the root and leaf tissues of seedlings exposed to Taunit, suggesting that MWCNTs have a capacity to penetrate the cell walls, accumulate in roots and translocate to the leaves. Thus the stimulating effect of MWCNTs on seedlings of may be associated with the primary uptake and accumulation of MWCNTs by plant roots followed by translocation to the other plant tissues.

关键词： multiwalled carbon nanotubes     plants     electron microscopy    

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Effects of nano-silicon and common silicon on lead uptake and translocation in two rice cultivars

Jianguo LIU,Hui CAI,Congcong MEI,Mingxin WANG

《环境科学与工程前沿（英文）》 2015年 第9卷 第5期   页码 905-911 doi: 10.1007/s11783-015-0786-x

摘要： The current study investigated the effects of nano-silicon (Si) and common Si on lead (Pb) toxicity, uptake, translocation, and accumulation in the rice cultivars Yangdao 6 and Yu 44 grown in soil containing two different Pb levels (500 mg·kg and 1000 mg·kg ). The results showed that Si application alleviated the toxic effects of Pb on rice growth. Under soil Pb treatments of 500 and 1000 mg·kg , the biomasses of plants supplied with common Si and nano-Si were 1.8%–5.2% and 3.3%–11.8% higher, respectively, than those of plants with no Si supply (control). Compared to the control, Pb concentrations in rice shoots supplied with common Si and nano-Si were reduced by 14.3%–31.4% and 27.6%–54.0%, respectively. Pb concentrations in rice grains treated with common Si and nano-Si decreased by 21.3%–40.9% and 38.6%–64.8%, respectively. Pb translocation factors (TFs) from roots to shoots decreased by 15.0%–29.3% and 25.6%–50.8%, respectively. The TFs from shoots to grains reduced by 8.3%–13.7% and 15.3%–21.1%, respectively, after Si application. The magnitudes of the effects observed on plants decreased in the following order: nano-Si treatment>common Si treatment and high-grain-Pb-accumulating cultivar (Yangdao 6)>low-grain-Pb-accumulating cultivar (Yu 44) and heavy Pb stress (1000 mg·kg )>moderate Pb stress (500 mg·kg )>no Pb treatment. The results of the study indicate that nano-Si is more efficient than common Si in ameliorating the toxic effects of Pb on rice growth, preventing Pb transfer from rice roots to aboveground parts, and blocking Pb accumulation in rice grains, especially in high-Pb-accumulating rice cultivars and in heavily Pb-polluted soils.

关键词： silicon (Si)     lead (Pb)     rice (Oryza sativa L.)     toxicity     accumulation    

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Influence and related mechanism of Retn gene expression on glucose uptake in 3T3-L1 cells

LI Yahui, DONG Shiyuan, YU Chao, JIANG Yu, LI Huaixing, SUN Shuhan

《医学前沿（英文）》 2007年 第1卷 第3期   页码 269-273 doi: 10.1007/s11684-007-0051-1

摘要： The aim of this article was to investigate the influence and the related mechanism of the gene on glucose uptake and insulin resistance in 3T3-L1 cells. Radioimmunoassay was used to determine glucose uptake in 3T3-L1 cells with different gene expression levels, whether cells were stimulated by insulin or not. RT-PCR and real-time RT-PCR analysis were used to determine the mRNA levels of several glucose transport proteins in 3T3-L1 cells with different gene expression levels, including insulin receptor substrate-1(IRS-1), phosphatidylinositol 3-kinase (PI-3K), AKT-2, glucose transporter-4 (GLUT-4), p38 mitogen-activated protein kinase (p38MAPK) and glycogen synthase kinase-3b (GSK-3). The glucose uptake decreased with the increase in gene expression in 3T3-L1 cells, which was independent of whether the cells were stimulated by insulin or not. The mRNA expression of two signal proteins PI-3K and AKT-2 decreased and the other two signal proteins, GSK-3 and p38MAPK, increased with overexpression in 3T3-L1 cells. Resistin could induce insulin resistance in adipocytes, which might be related to the changes of some proteins in PI-3K and Ras pathways.

关键词： 3T3-L1     influence     resistance     receptor substrate-1     transport    

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Interface engineering for enhancing electrocatalytic oxygen evolution reaction of CoS/CeO heterostructures

《化学科学与工程前沿（英文）》 2022年 第16卷 第3期   页码 376-383 doi: 10.1007/s11705-021-2062-x

摘要： To realize renewable energy conversion, it is important to develop low-cost and high-efficiency electrocatalyst for oxygen evolution reaction. In this communication, a novel bijunction CoS/CeO2 electrocatalyst grown on carbon cloth is prepared by the interface engineering. The interface engineering of CoS and CeO2 facilitates a rapid charge transfer from CeO2 to CoS. Such an electrocatalyst exhibits outstanding electrocatalytic activity with a low overpotential of 311 mV at 10 mA∙cm−2 and low Tafel slope of 76.2 mV∙dec–1, and is superior to that of CoS (372 mV) and CeO2 (530 mV) counterparts. And it has long-term durability under alkaline media.

关键词： interface engineering     CoS/CeO2     electrodeposition     electrocatalyst     oxygen evolution reaction    

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High-entropy catalysts for electrochemical water-electrolysis of hydrogen evolution and oxygen evolution

《能源前沿（英文）》 doi: 10.1007/s11708-023-0892-6

摘要： High entropy materials (HEMs) have developed rapidly in the field of electrocatalytic water-electrolysis for oxygen evolution reaction (OER) and hydrogen evolution reaction (HER) due to their unique properties. In particular, HEM catalysts are composed of many elements. Therefore, they have rich active sites and enhanced entropy stability relative to single atoms. In this paper, the preparation strategies and applications of HEM catalysts in electrochemical water-electrolysis are reviewed to explore the stabilization of HEMs and their catalytic mechanisms as well as their application in support green hydrogen production. First, the concept and four characteristics of HEMs are introduced based on entropy and composition. Then, synthetic strategies of HEM catalysts are systematically reviewed in terms of the categories of bottom-up and top-down. The application of HEMs as catalysts for electrochemical water-electrolysis in recent years is emphatically discussed, and the mechanisms of improving the performance of electrocatalysis is expounded by combining theoretical calculation technology and ex-situ/in situ characterization experiments. Finally, the application prospect of HEMs is proposed to conquer the challenges in HEM catalyst fabrications and applications.

关键词： high-entropy     electrocatalysis     synthetic methods     water-electrolysis     hydrogen and oxygen evolutions    

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标题 作者 时间 类型 操作

Effect of short-term atrazine addition on the performance of an anaerobic/anoxic/oxic process

Changyong WU, Xiaoling LI, Zhiqiang CHEN, Yongzhen PENG,

期刊论文

Reduction of wastewater toxicity and change of microbial community in a hydrolysis acidification reactor pre-treating trimethylolpropane wastewater

Xin Xing, Yin Yu, Hongbo Xi, Guangqing Song, Yajiao Wang, Jiane Zuo, Yuexi Zhou

期刊论文

the addition of organic carbon sources on nitrous oxide emission in anaerobic-aerobic (low dissolved oxygen

Hongjing LI, Xiurong CHEN, Yinguang CHEN

期刊论文

Comments on “Prediction on CO uptake of recycled aggregate concrete”, Frontiers of Structural and Civil

期刊论文

Organic and inorganic phosphorus uptake by bacteria in a plug-flow microcosm

Jinbo ZHAO, Xuehua LIU

期刊论文

The implications of planting mode on cadmium uptake and remobilization in rice: Field experiments across

期刊论文

Denitrification and phosphorus uptake by DPAOs using nitrite as an electron acceptor by step-feed strategies

Bin MA, Shuying WANG, Guibing ZHU, Shijian GE, Junmin WANG, Nanqi Ren, Yongzhen PENG

期刊论文

Effects of nitrite on phosphate uptake in anaerobic-oxic process

LI Jie, XIONG Biyong, ZHANG Shude, YANG Hong, ZHANG Jie

期刊论文

Design of nanocarriers for efficient cellular uptake and endosomal release of small molecule and nucleic

Vaibhav Mundra, Ram I. Mahato

期刊论文

Heterometallic cluster-based organic frameworks as highly active electrocatalysts for oxygen reductionand oxygen evolution reaction: a density functional theory study

期刊论文

Uptake and accumulation of multiwalled carbon nanotubes change the morphometric and biochemical characteristics

Elena SMIRNOVA, Alexander GUSEV, Olga ZAYTSEVA, Olga SHEINA, Alexey TKACHEV, Elena KUZNETSOVA, Elena LAZAREVA, Galina ONISHCHENKO, Alexey FEOFANOV, Mikhail KIRPICHNIKOV

期刊论文

Effects of nano-silicon and common silicon on lead uptake and translocation in two rice cultivars

Jianguo LIU,Hui CAI,Congcong MEI,Mingxin WANG

期刊论文

Influence and related mechanism of Retn gene expression on glucose uptake in 3T3-L1 cells

LI Yahui, DONG Shiyuan, YU Chao, JIANG Yu, LI Huaixing, SUN Shuhan

期刊论文

Interface engineering for enhancing electrocatalytic oxygen evolution reaction of CoS/CeO heterostructures

期刊论文

High-entropy catalysts for electrochemical water-electrolysis of hydrogen evolution and oxygen evolution

期刊论文